J. Morel et al., EMISSION PROBABILITIES OF L X-, K X- AND GAMMA-RAYS IN THE 10-130 KEVRANGE FOLLOWING THE DECAY OF PU-239, Nuclear instruments & methods in physics research. Section A, Accelerators, spectrometers, detectors and associated equipment, 339(1-2), 1994, pp. 232-240
X- and gamma-ray emission probabilities in the 10-130 keV range were a
ccurately measured for Pu-239 using calibrated Ge detectors. Data belo
w 60 keV are essential for the development of environmental and contam
ination measurement techniques; data above 60 keV are required mainly
for nondestructive analyses applicable to nuclear material safeguards.
X- and gamma-ray spectra were obtained from an electroplated Pu-239 s
ource With an activity of 0.5 MBq using calibrated collimated planar-G
e and coaxial-Ge detectors. An additional electroplated source of 3 MB
q Pu-239 was counted to improve the spectrum analysis in the K X-ray r
egion. L and K X-ray peaks were fitted to Voigt functions while gamma-
ray peaks were described by Gaussian functions; anomalous K X-ray line
shapes were observed from the decay of Pu-239. The principal X- and g
amma-ray emission probabilities were determined with an uncertainty of
1% or better. For example, the following results were obtained for Pu
-239: L(total) X-rays = (4.67 +/- 0.05) X 10(-2), K-alpha X-rays = (1.
219 +/- 0.009) X 10(-4), 38.7 keV gamma-ray = (1.044 +/- 0.013) X 10(-
4) and 129.3 keV gamma-ray = (6.31 +/- 0.03) X 10(-5).