Excitation of surface phonons or surface acoustic wave (SAW) pulses wi
th a broad frequency spectrum up to 200-300 MHz using focused laser pu
lses is discussed. Several optical and piezoelectric methods for broad
band detection of the resulting surface displacements are considered.
It is shown that for an anisotropic single crystal the SAW velocity ca
n be measured with an accuracy of 0.1% as a function of the crystal pl
ane and direction due to the short wave pulses achieved. In a layered
system strong dispersion occurs, since the waves with different wavele
ngths probe different depths corresponding to their wavelength and thu
s travel with different velocities in the. heterogeneous solid. From a
non-linear dispersion effect several film properties can be obtained,
such as thickness, density and elastic constants (e.g, Young's modulu
s and Poisson's ratio). Results are presented for fullerite and diamon
dlike carbon films. The characteristics of the pulsed laser method are
compared with Brillouin scattering, interdigital transducers and the
acoustic microscope.