ON THE PREPARATION AND MEASUREMENT OF SUPERPOSITIONS OF CHIRAL AMPLITUDES

Authors
Citation
Ja. Cina et Ra. Harris, ON THE PREPARATION AND MEASUREMENT OF SUPERPOSITIONS OF CHIRAL AMPLITUDES, The Journal of chemical physics, 100(4), 1994, pp. 2531-2536
Citations number
16
Categorie Soggetti
Physics, Atomic, Molecular & Chemical
ISSN journal
00219606
Volume
100
Issue
4
Year of publication
1994
Pages
2531 - 2536
Database
ISI
SICI code
0021-9606(1994)100:4<2531:OTPAMO>2.0.ZU;2-5
Abstract
We examine the preparation and detection of superpositions of chiral a mplitudes of a handed molecule, showing that specific sequences of pha se-controlled ultrashort light pubes enable the preparation and measur ement of chiral coherences. It is found that certain choices of relati ve optical phase between the pulses of the preparation sequence set up left-right superpositions that would be inaccessible by tunneling dyn amics alone.