Ja. Cina et Ra. Harris, ON THE PREPARATION AND MEASUREMENT OF SUPERPOSITIONS OF CHIRAL AMPLITUDES, The Journal of chemical physics, 100(4), 1994, pp. 2531-2536
We examine the preparation and detection of superpositions of chiral a
mplitudes of a handed molecule, showing that specific sequences of pha
se-controlled ultrashort light pubes enable the preparation and measur
ement of chiral coherences. It is found that certain choices of relati
ve optical phase between the pulses of the preparation sequence set up
left-right superpositions that would be inaccessible by tunneling dyn
amics alone.