The Concentration-Controlled Recycle Reactor. The scope offered by the
concentration-controlled recycle reactor for elucidating the kinetics
of heterogeneous gas reactions is. presented in three contexts: ident
ification of reaction networks; experimental design; and separate dete
rmination of changes of activity. Control strategies appropriate for t
he problem at hand are an essential prerequisite for the application o
f experimental strategies. In particular, long analysis cycles require
appropriate modification of modern methods of control theory. Various
model-based control concepts have been developed and tested by experi
ment and simulation.