B. Ji et al., FINAL-STATE ALIGNMENT FROM THE QUANTUM-STATE-SELECTED PHOTODISSOCIATION OF K-2 BY ALL-OPTICAL TRIPLE-RESONANCE SPECTROSCOPY, Physical review. A, 49(3), 1994, pp. 180001535-180001538
We have measured the final atomic excited-state alignment following th
e quantum-state-selected photodissociation of K2 through quasibound ro
tational resonance states using cw all-optical triple resonance spectr
oscopy. This process constitutes the half-collision analog of K + K s
cattering through a precisely quantum-state-selected orbiting resonanc
e. The final atomic-state alignment depends sensitively on the parity
of the excited continuum state. The experimental results show excellen
t agreement with theoretical calculations.