Ji. Dadap et al., RANDOMLY ORIENTED ANGSTROM-SCALE MICROROUGHNESS AT THE SI(100) SIO2 INTERFACE PROBED BY OPTICAL 2ND-HARMONIC GENERATION, Applied physics letters, 64(16), 1994, pp. 2139-2141
Femtosecond pulses from a Kerr-Lens mode-locked Ti:sapphire laser are
used to generate second harmonic from a series of native-oxidized Si(1
00)/SiO2 and hydrogen-terminated Si(100) samples prepared with systema
tically varied interfacial microroughness with root-mean-square featur
e heights ranging from 0.6 to 4.3 angstrom. Rotationally anisotropic s
econd harmonic signals using different polarization configurations wer
e measured in air and correlated with atomic force microscopy measurem
ents. The results demonstrate rapid, noncontact, noninvasive measureme
nt of Angstrom-level Si(100)/SiO2 interface roughness by optical secon
d harmonic generation.