Pd. Wang et al., PHOTOLUMINESCENCE INTENSITY AND MULTIPLE PHONON RAMAN-SCATTERING IN QUANTUM DOTS - EVIDENCE OF THE BOTTLENECK EFFECT, Surface science, 305(1-3), 1994, pp. 585-590
We report a systematic study of photoluminescence efficiency in dry et
ched quantum well dots. Luminescence degradation is observed on decrea
sing the quantum dot lateral size. Furthermore, luminescence quenching
is more pronounced in quantum dots with a thicker quantum well than t
hose with a thinner one. This effect is attributed to the reduced carr
ier relaxation in 0D system. Resonant Raman scattering and ''hot'' exc
iton luminescence have also been observed in dry etched GaAs/AlGaAs qu
antum dots in which quantum confinement effects are found with decreas
ing dot sizes. Up to 4th-order multiphonon processes have been observe
d through photoluminescence and photoluminescence excitation in quantu
m dots. These results are direct evidence of the bottleneck effect. La
teral patterning of quantum wells strongly localises excitons in three
-dimensional quantum confinement regime (0D system). The observation o
f resonant Raman scattering and hot exciton luminescence up to high te
mperature demonstrates the high stability of localised excitons.