Wt. Coffey et al., EXACT ANALYTIC FORMULA FOR THE CORRELATION TIME OF A SINGLE-DOMAIN FERROMAGNETIC PARTICLE, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics, 49(3), 1994, pp. 1869-1882
Exact solutions for the longitudinal relaxation time T(parallel-to) an
d the complex susceptibility chi(parallel-to)(omega) of a thermally ag
itated single-domain ferromagnetic particle are presented for the simp
le uniaxial potential of the crystalline anisotropy considered by Brow
n [Phys. Rev. 130, 1677 (1963)]. This is accomplished by expanding the
spatial part of the distribution function of magnetic-moment orientat
ions on the unit sphere in the Fokker-Planck equation in Legendre poly
nomials. This leads to the three-term recurrence relation for the Lapl
ace transform of the decay functions. The recurrence relation may be s
olved exactly in terms of continued fractions. The zero-frequency limi
t of the solution yields an analytic formula for T(parallel-to) as a s
eries of confluent hypergeometric (Kummer) functions which is easily t
abulated for all potential-barrier heights. The asymptotic formula for
T(parallel-to) of Brown is recovered in the limit of high barriers. O
n conversion of the exact solution for T(parallel-to) to integral form
, it is shown using the method of steepest descents that an asymptotic
correction to Brown's high-barrier result is necessary. The inadequac
y of the effective-eigenvalue method as applied to the calculation of
T(parallel-to) is discussed.