Ferromagnetic thin films of La2-2xCa1+2xMn2O7 (x=0.3) with a tetragona
l Sr3Ti2O7-type layered perovskite structure have been deposited on Mg
O and SrTiO3 (001) substrates by magnetron sputtering. The epitaxial t
hin films in this study have the a-axis normal orientation with 90 deg
rees domains having the a/c boundaries in the film plane. These thin f
ilms exhibit highly enhanced magnetoresistance (MR) effects (MR ratio
Delta rho/rho(0) of -93% at mu(0)H=1T) compared with those reported fo
r thin films of cubic ferromagnetic perovskite with isotropic Mn-O net
works. These MR behavior can be explained by taking account of the two
-dimensionality and anisotropy of the Mn-O networks in the ferromagnet
ic layered perovskites.