Ys. Zeng et Pk. Hopke, COMPARISON OF THE SOURCE LOCATIONS AND SEASONAL PATTERNS FOR ACIDIC SPECIES IN PRECIPITATION AND AMBIENT PARTICLES IN SOUTHERN ONTARIO, CANADA, Science of the total environment, 143(2-3), 1994, pp. 245-260
The Potential Source Contribution Function (PSCF) is a probability fun
ction based on the air parcel trajectory data coupled with information
regarding the nature of the contaminants measured in that air parcel.
The PSCF value is the ratio of the probability of a contaminated air
parcel having traversed a 1-degrees latitude by 1-degrees longitude ar
ea to the probability that any air parcel traversed that area. Regions
with high PSCF values thus have a higher probability of contributing
pollutants to the measured concentrations at the receptor site. Previo
usly, PSCF analysis has been used on precipitation chemistry data obta
ined from the Acidic Precipitation in Ontario Study (APIOS) to locate
the sources of the acidic precipitation. In this present study, the me
thodology has been applied to both precipitation samples and particula
te samples collected by the APIOS network. Analyses have been performe
d separately for the winter and summer seasons so that the comparison
between particles and precipitation and/or winter and summer can be ma
de. From these results it is possible to identify the possible source
locations for the observed constituents and at the same time, derive i
nformation on atmospheric process by this study.