P. Carretta et al., SPIN DYNAMICS IN A 2-DIMENSIONAL DISORDERED S=1 2 HEISENBERG PARAMAGNET FROM CU-63 NQR RELAXATION IN ZN-DOPED LA2CUO4/, Physical review. B, Condensed matter, 55(6), 1997, pp. 3734-3741
Cu-63 NQR T-1 and T-2 relaxation measurements in La2Cu1-xZnxO4, for 0
less than or equal to x less than or equal to 0.11 and in the temperat
ure range T-N less than or equal to T less than or equal to 900 K, are
presented. The results are used to derive insights into the Cu2+ corr
elated spin dynamics in the paramagnetic phase of the S=1/2 two-dimens
ional (2D) Heisenberg (H) antiferromagnets (AF), and into the disorder
effects associated with the spin vacancy due to Zn2+ (S=0) for Cu2+ s
ubstitution. In particular, by using scaling arguments for the static
generalized susceptibility, chi(-->(q),0), and for the decay rate, Gam
ma-->(q), of the normal excitations, T-2 and T-1 are related to the in
-plane correlation length xi(2D)(x,T) and its dependence on temperatur
e and Zn doping, x, is extracted. The experimental findings are analyz
ed in light of the quantum critical and renormalized classical behavio
rs for xi(2D) predicted by recent theories for S=1/2 HAF on square lat
tices. It is shown that up to T similar or equal to 900 K, xi(2D) is c
onsistent with the assumption of a renormalized classical regime, in a
greement with recent neutron scattering results and at variance with p
revious interpretations of the NQR data. It is discussed how Zn affect
s xi(2D) through the modification in the spin stiffness and comparison
with the disorder induced by itinerant extra holes is made.