Vi. Klimov et al., NONLINEAR-TRANSMISSION SPECTRA OF POROUS SILICON - MANIFESTATION OF SIZE QUANTIZATION, Applied physics letters, 64(20), 1994, pp. 2691-2693
Changes in the transmission of porous silicon layers induced by ultras
hort laser pulses are studied by using picosecond pump and probe measu
rements. Bleaching bands attributed to the saturation of optical trans
itions in silicon wires or/and crystallites with nanometer dimensions
are observed in time-resolved differential transmission spectra. The m
easured nonlinearity is characterized by a relatively high value of th
e third-order nonlinear susceptibility (almost-equal-to 10(-8) esu) an
d by fast relaxation dynamics (transmission recovery time is 30-40 ps)
.