E. Glikman et al., ELEMENTAL AND ISOTOPIC EFFECTS IN NEUTRON-INDUCED DESORPTION FROM SURFACES, Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms, 88(3), 1994, pp. 237-243
Recoil of atoms following (n, gamma) reactions may cause them to desor
b from the surface. This effect is studied in irradiation experiments
under high thermal neutron flux for gold and iridium, utilizing prepac
kaged ampules under vacuum. The role of thermal desorption is demonstr
ated, through a comparative study of the behavior of different element
s under identical conditions. Precise measurements of the populations
of iridium isotopes were carried out, revealing large Ir-194/Ir-192 di
fferentiation. This is shown to be related to the temporal history of
desorption during the irradiation, and provides additional meaningful
information about the process.