High-resolution optical stellar and interstellar observations toward t
he halo star HD 203664 and six surrounding early-type stars have been
combined with a 21 cm mapping of the region to investigate a 70 km s-1
high-velocity cloud (HVC). The distance of the HVC from the Galactic
plane (z) has been constrained to lie between 200 and 1500 pc; upper l
imits to temperature and velocity dispersion of 4600 K and 2.2 km s-1
have been estimated; and a column density ratio N(Na II)/N(Ca II) cong
ruent-to 0.32 has been deduced. These parameters are consistent with t
he material being shocked gas, possibly arising from an old supernova
remnant. The N(Na I)/N(H I) and N(Ca II)/N(H I) ratios are anomalously
large by factors of approximately 20 and 100, respectively, with resp
ect to normal diffuse gas; several scenarios are presented as possible
explanations of this phenomenon.