The structural and magnetic properties of YFe10-xCoxMo2 alloys (0 less
-than-or-equal-to x less-than-or-equal-to 10) have been investigated b
y means of x-ray diffraction, thermomagnetic analysis, and magnetometr
y techniques. All the alloys exhibited the tetragonal ThMn12 structure
and were almost single phase materials. With the increase of Co conte
nt x, T(c) increases initially, reaching a maximum at x approximately
6, followed by a decrease at higher x values. X-ray diffraction analys
es on magnetically aligned samples indicate that YFe10Mo2 exhibits an
axial easy direction of magnetization (EDM) at room temperature, and t
he addition of Co initially causes the EDM to deviate gradually from t
he c axis with increasing x (x less-than-or-equal-to 4). On further in
crease of Co content (x greater-than-or-equal-to 5), the EDM of the YF
e10-xCoxMo2 compounds tends to become axial again, reaching a complete
uniaxial behavior for the terminal compound YCo10Mo2.