Fast photography with a framing streak camera is applied to investigat
e the dynamics of ablated Fe particles by a pulsed excimer laser when
a nitrogen atmosphere is present. Two stages of expansion are found in
the generated plume. The first one starts just after the laser irradi
ation where the hemispherical and unidirectional plumes are found simu
ltaneously. The dynamics of the unidirectional plume is described by a
drag model for 300 ns. The second stage occurs at 300 ns, and the uni
directional plume expands again in agreement with a delayed blast wave
model. The thickness distribution of the deposited Fe-N film is well
correlated with the change in the plume geometry, then with the nitrog
en pressure.