Tr. Thurston et al., X-RAY-SCATTERING AND NEUTRON-SCATTERING MEASUREMENTS OF 2 LENGTH SCALES IN THE MAGNETIC CRITICAL FLUCTUATIONS OF HOLMIUM, Physical review. B, Condensed matter, 49(22), 1994, pp. 15730-15744
The short-ranged correlations associated with magnetic ordering in the
rare-earth antiferromagnet holmium have been characterized in high-re
solution x-ray- and neutron-scattering studies. For temperatures withi
n about 2 K above T(N), the short-ranged magnetic fluctuations exhibit
two length scales, instead of the single one expected in an ideal sys
tem. Well above T(N), the shorter of the two length scales exhibits po
wer-law behavior consistent with normal critical fluctuations; the lin
e shape in momentum space is well described by a Lorentzian, and the m
easured critical exponents are nu=0.54+/-0.04 and gamma=1.24+/-0.15. T
he longer of the two length scales is well described by a squared-Lore
ntzian line shape, and exhibits a power-law temperature dependence. Bo
th the shorter and the longer length-scale fluctuations are approximat
ely spatially isotropic. We propose that the longer length-scale fluct
uations are related to random strain fields which are localized at or
near the sample surfae. These results are reminiscent of behavior obse
rved at the cubic-to-tetragonal structural phase transitions of some p
erovskite materials.