Scanning electron microscopy with polarization-analysis (SEMPA) measur
ements of the dependence of the oscillations of the exchange coupling
in Fe/Cr/Fe(100) structures on the Cr growth temperature are correlate
d with the thickness fluctuations in Cr films measured by scanning tun
neling microscopy (STM) at similar growth temperatures. Layer-by-layer
growth was observed by STM for Cr deposition on very flat Fe(100) whi
skers at deposition temperatures greater-than-or-equal-to 300-degrees-
C. The SEMPA measurements of the magnetization of the Fe overlayer as
a function of Cr spacer-layer thickness at this temperature could be s
imulated well by oscillatory coupling with periods 2.105+/-0.005d and
12+/-1d, where d is the layer spacing. Rougher Cr growth, limited by d
iffusion kinetics, occurs at lower growth temperatures giving a distri
bution of thicknesses in the growth front as determined by STM. We mod
eled the Fe magnetization for lower-temperature Cr growth by assuming
that the exchange coupling at each discrete Cr thickness is the same a
s found for layer-by-layer growth. The total coupling at each average
Cr spacer-layer thickness was determined by adding the weighted contri
bution to the coupling from each Cr layer thickness contributing to th
e average thickness. Thus, by taking into account the thickness fluctu
ations in the Cr spacer layer as determined by STM, very good agreemen
t was obtained between the model and the SEMPA measurement of the Fe o
verlayer magnetization for Cr growth at lower temperatures without inc
luding other consequences of roughness at the interface, such as the b
reakdown of translational invariance. Important characteristic length
scales and the role of biquadratic coupling in the SEMPA measurements
are addressed.