G. Korschinek et al., AMS FOR M-GREATER-THAN-36 WITH A GAS-FILLED MAGNETIC SPECTROGRAPH, Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms, 92(1-4), 1994, pp. 146-152
Small concentrations of long-lived radioisotopes such as Ni-59 are not
necessarily easy to determine by AMS because of the background of sta
ble isobars, in this case Co-59. The gas-filled Q3D magnetic spectrogr
aph has been successfully used for isobaric separation. Additional sup
pression of non-isobaric background is accomplished by means of a Wien
filter directly after the tandem and a highly sensitive time-of-fligh
t measurement just before the spectrograph. Until now we have used the
se techniques for the radioisotopes Ca-41, Ni-59, Sr-90 and Pd-107. Th
e limits in sensitivity am at present between approximately 3 x 10(-15
) for Ca-41/Ca and approximately 1 x 10(-8) for Pd-107/Pd-106. Measure
ments have been performed on environmental, extraterrestial and nuclea
r waste samples. Because of the insufficient sensitivity for measureme
nts of very low concentrations with the existing Q3D, a dedicated gas-
filled magnet with a deflection angle of 135-degrees is now under cons
truction.