H. Artigalas et al., APPLICATION OF AMS AND INVERSE PIXE TO THE STUDY OF RADIOACTIVE-WASTEMANAGEMENT PROBLEMS, Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms, 92(1-4), 1994, pp. 227-230
Some long-lived radionuclides (Ni-59, Zr-93, Mo-93, Nb-94, Tc-99, Pd-1
07, Sm-151) must be measured at levels < 10(-3) Bq/g in radioactive wa
stes. No method is able to achieve this at the moment, except accelera
tor mass spectrometry (AMS) in the case of Ni-59, using high energies.
In this paper, we show that AMS at low energy (with a 3 MV tandem) is
in principle able to measure the radionuclides of interest with the r
equired sensitivity. To overcome the isobaric interferences, which are
the limiting factor in AMS, characteristic projectile X-rays are meas
ured (''inverse PIXE'').