Nuclear magnetic resonance (NMR) and low-temperature magnetization mea
surements are used to demonstrate antiferromagnetic (AF) coupling in m
olecular beam epitaxy grown (111)-oriented Co/Pt superlattices. Drasti
c changes in the NMR spin-echo spectra as a function of the in-plane d
c magnetic-field strength provide conclusive evidence of AF interlayer
coupling in these structures, consisting of 35- and 52-angstrom Co an
d 18-angstrom Pt bilayers. The structure of the Co films is mainly hcp
(70%) and the coupling energy per unit area, as determined from in-pl
ane magnetization loops is found to range up to 1 erg/cm2.