S. Whitlow et al., AN ICE-CORE-BASED RECORD OF BIOMASS BURNING IN THE ARCTIC AND SUB-ARCTIC, 1750-1980, Tellus. Series B, Chemical and physical meteorology, 46(3), 1994, pp. 234-242
Ammonium records from 3 ice cores, 20D and GISP2 (Greenland) and Mt. L
ogan (Yukon), covering the period from 1750 to the 1980s are analyzed.
For each data set, samples with NH4+ concentrations greater than one
standard deviation above the mean value also tend to be enriched in NO
3- and K+, similar to the chemical composition of aerosols from aged b
iomass burning plumes. We believe the NH4+ spikes originate from bioma
ss burning events. There is not a one to one correspondence between do
cumented large fires and NH4+ spikes, nor are specific annual layers w
ith elevated NH4+ concentrations often found in more than one core. Ho
wever, frequency of NH4+ spikes increase during periods of more extens
ive and intensive biomass burning in the NH4+ source areas for the ice
core sites. The 20D and GISP2 records are characterized by increased
spike frequency from 1790 to 1810 and from 1830 to 1910. This latter t
ime coincides with a period of increased biomass burning documented in
the historical fire records for northern North America. In contrast t
o both Greenland ice core records, the Mt. Logan NH4+ record shows per
iods of increased spike frequency from 1770-1790, 1810-1830, 1850-1870
and 1930-1980. The poor agreement between the Mt. Logan record and th
e records from Greenland suggests that another source area, perhaps Si
beria, may be the dominant summertime source area for NH4+ spikes in M
t. Logan snow.