T. Starczewski et al., TIME-RESOLVED HARMONIC-GENERATION IN AN IONIZING GAS, Journal of physics. B, Atomic molecular and optical physics, 27(14), 1994, pp. 3291-3301
We report on a time-resolved study of the fifth harmonic generated in
xenon by 140 ps pulses from a Nd:YAG laser in the 10(13) W cm-2 intens
ity regime. Absolute timing between the driving laser pulse and the ha
rmonic pulse could be determined by means of reference harmonics gener
ated in non-linear crystals and a single common streak camera. Above a
certain laser intensity the centre of the observed harmonic pulse was
shifted earlier in time relative to the laser pulse. We found the int
ensity dependence of this shift to be approximately linear within the
intensity range used which is consistent with the results of numerical
simulations taking the ionization and dispersion of the xenon gas int
o account.