C. Garrigoulagrange et al., INELASTIC ELECTRON-TUNNELING SPECTROSCOPY OF BIS(ETHYLENEDITHIO)TETRATHIAFULVALENE (BEDT-TTF) COMPOUNDS, Chemical physics letters, 225(4-6), 1994, pp. 297-302
Inelastic electron tunneling spectra of thin films of bis(ethylenedith
io)tetrathiafulvalene (BEDT-TTF) and its salts: a low temperature supe
rconductor K-(BEDT-TTF)2Cu(NCS)2 and an insulator (BEDT-TTF)2Mo6O19 ar
e measured at 4.2 K in the range 230-1650 cm-1 and compared with infra
red spectra of the same compounds at room temperature. The obtained vi
brational bands are assigned following theoretical normal mode calcula
tions. Electron-molecular vibration coupling theory of charge-transfer
organic compounds is extended to the case of electron tunneling spect
ra.