MuLCR spectra from single-crystal Si:Al have been taken at 30 K with t
he field along the [111] direction. The spectra show strong resonances
near 12 and 50 mT, and weaker resonances near 38 and 42 mT. There is
also indication of lines near 15 and 21 mT. The strong signals are due
to the well-known zero crossings for Mu in Si, and the weak signals
may be associated with the quadrupole interaction of Al-27, as predict
ed by ab initio electronic structure calculations.