We have performed several physical and optical measurements on the Cr:
LiSAF (LiSrAlF6) laser material that are relevant to its laser perform
ance, including thermal and mechanical properties, water durabilities,
and Auger upconversion constants. The expansion coefficient, Young's
modulus, fracture toughness, thermal conductivity, and heat capacity a
re all used to determine an overall thermomechanical figure of merit f
or the crystal. An investigation of the water durability suggests that
the cooling solution should be maintained at pH = 7 to ameliorate pro
blems associated with water dissolution. The Auger constant was found
to become much more significant at higher Cr doping, in which excited-
state migration leads to a substantial increase in the upconversion ra
te. We propose a design for a 50-W Cr:LiSAF laser system that is based
on a detailed knowledge of all the relevant material parameters.