SPIN FLUCTUATIONS IN DOPED ANTIFERROMAGNETS FROM LI-7 NMR RELAXATION IN CUOLI

Citation
P. Carretta et al., SPIN FLUCTUATIONS IN DOPED ANTIFERROMAGNETS FROM LI-7 NMR RELAXATION IN CUOLI, Physical review. B, Condensed matter, 49(10), 1994, pp. 7044-7047
Citations number
22
Categorie Soggetti
Physics, Condensed Matter
ISSN journal
01631829
Volume
49
Issue
10
Year of publication
1994
Pages
7044 - 7047
Database
ISI
SICI code
0163-1829(1994)49:10<7044:SFIDAF>2.0.ZU;2-M
Abstract
Li-7 NMR relaxation is used to derive information on the low-energy sp in excitations induced in antiferromagnetic (AF) CuO by the heterovale nt substitution of one percent of Cu2+ by Li+. The energy gap E(g) bet ween localized and itinerant states, where the extra hole diffuses in the AF matrix, is obtained as E(g) congruent-to 600 K while the effect ive correlation time of the hole is tau(h) congruent-to (1/omega(exch) /xe(-E(g)/T), in agreement with the main conclusions of a previous wor k in Cu1-xLixO for larger doping [P. Carretta, M. Corti, and A. Rigamo nti, Phys. Rev. B 48, 3433 (1993)]. The experimental findings are disc ussed in comparison with the ones in lightly doped AF La2-xSrxCuO4, wh ere a drastic changeover in the x dependence of the spin fluctuation p roperties has been recently found for x less than or similar to 0.02 [ F. C. Chou et al., Phys. Rev. Lett. 71, 2323 (1993)]. Finally, mostly on the basis of Li-7 relaxation rates at different measuring frequenci es, it is conjectured that in Cu0.99Li0.01O one has a localization of the extra hole, possibly in the CuO4 plaquette [R. J. Gooding, Phys. R ev. Lett. 66, 2266 (1991)], establishing a condition of fast spin fluc tuations.