This paper considers the design of multistage membrane plants operatin
g in the diffusion controlled region where gas flux is proportional to
the differences in the gas partial pressure across the membrane. The
flow inside the modular stages was assumed to be fully mixed and the s
tages were connected in a simple countercurrent mode. The design metho
d was thus particularly aimed at separations involving inorganic membr
anes. A flexible algorithm was used to define the interstage flow sequ
ence and the plant was assumed to be built of modules of the same size
; only the number of modules assigned to a stage was allowed to vary.
Trial and error was used to obtain convergence of the plant mass balan
ce. The criteria for optimisation are discussed. Predictions of module
behaviour for the fully mixed and the more realistic plug flow cases
are considered in an appendix. Based on this comparison, the applicabi
lity of the current design methods for stage cuts above 0.2 is questio
nable.