Aa. House et al., THE LOW-TEMPERATURE PHASE OF ALPHA-(BEDT-TTF)(2)KHG(SCN)(4) .2. PRESSURE-DEPENDENCE OF THE SHUBNIKOV-DEHAAS OSCILLATIONS, Journal of physics. Condensed matter, 8(49), 1996, pp. 10377-10392
The magnetoresistance of alpha-(BEDT-TTF)(2)MHg(SCN)(4) (where BEDT-TT
F is bis(ethylenedithio)tetrathiafulvalene and M = NH4 or K) has been
studied under pressures of up to 14.8 kbar and for temperatures down t
o 0.7 K. The similar to 671 T (alpha) and similar to 4270 T (beta) Shu
bnikov-de Haas oscillations observed in the ambient pressure magnetore
sistance of alpha-(BEDT-TTF)(2)KHg(SCN)(4) persist to the highest pres
sure while the other quantum oscillatory frequencies are removed under
pressure. A strong second-harmonic component of the alpha-frequency o
scillations is observed on the raw data at 1 bar and is initially supp
ressed by pressure but returns above similar to 9 kbar. Furthermore, i
n the salt alpha-(BEDT-TTF)(2)NH4Hg(SCN)(4) a similar pronounced secon
d harmonic of the quantum oscillations has been observed at the highes
t pressures. The origins of these features of the data are discussed i
n the context of current models of the Fermi surfaces of these materia
ls.