Rn. Scoon et Aa. Mitchell, DISCORDANT IRON-RICH ULTRAMAFIC PEGMATITES IN THE BUSHVELD COMPLEX AND THEIR RELATIONSHIP TO IRON-RICH INTERCUMULUS AND RESIDUAL LIQUIDS, Journal of Petrology, 35(4), 1994, pp. 881-917
The iron-rich ultramafic pegmatities comprise a suite of coarse-graine
d rocks that form discordant bodies within the layered sequence of the
Bushveld Complex. These pegmatities, which are considerably more abun
dant than is generally realized, provide evidence for the differentiat
ion of iron-rich residual melts. The pegmatities are composed largely
of iron-rich olivine and clinopyroxene, together with Ti-magnetite and
ilmenite. Feldspar is characteristically absent, but paradoxically th
e pegmatities preferentially replace anorthositic cumulates. Two subgr
oups are recognized, olivine-clinopyroxene pegmatite and Fe-Ti oxide p
egmatite. With increased stratigraphic height the pegmatities become r
icher in Fe-Ti oxides. Thus, olivine-clinopyroxene pegmatite is preval
ent in the Upper Critical and Lower Main Zones, whereas Fe-Ti oxide pe
gmatite is restricted to the Upper Main and Upper Zones. Zoned pegmati
te, with a core of Fe-Ti oxide pegmatite, is transitional between the
two subgroups. New whole-rock and electron microprobe analyses of oliv
ine-clinopyroxene pegmatite from the Upper Critical and Lower Main Zon
es provide convincing evidence that their composition is directly rela
ted to height. Cryptic compositional variations are analogous to those
displayed by the layered cumulates, but for a given height the pegmat
ites are always more evolved. Compositions of clinopyroxene in the peg
matites reflect a near-linear relationship with height, whereas cumulu
s pyroxenes display upward iron-enrichment trends complicated by reple
nishment and reaction with trapped intercumulus liquid. The olivine-cl
inopyroxene pegmatite formed by magmatic replacement of earlier-formed
cumulates in response to infiltration of iron-rich melts. Suitably di
fferentiated melts comprised intercumulus and residual liquids derived
from thick anorthosite layers. The absence of feldspar, although not
fully understood, is attributed to an immiscible relationship between
dense, iron-rich melts and light, silica-alkali-rich liquids. The latt
er infiltrated upward to be reincorporated into the resident magma. Th
e iron-rich melts, however, drained down into the crystallizing cumula
te pile. Channelling along early-formed fractures and joints was signi
ficant, locally resulting in huge pipe-like bodies of pegmatite. The i
ron-rich melts became increasingly differentiated with height, partly
in response to the fractional crystallization of more evolved cumulate
s. The olivine-clinopyroxene pegmatites are related to infiltration of
Fe-Ti oxide-rich silicate melt, whereas Fe-Ti oxide pegmatite is ascr
ibed to Fe-Ti oxide liquid, as originally argued by Bateman (1951). Th
e Bushveld Complex followed the Fenner trend of almost uninterrupted i
ron enrichment. Evidence of pronounced iron enrichment is, however, ma
nifested in the discordant iron-rich ultramafic pegmatites several tho
usands of metres below the height at which iron-rich cumulates are obs
erved.