Compounds in the series Sm2Fe14-xCoxAl3 (x = 0, 1, 2, 3, 4 and 5) have
been shown to be of the Th2Zn17 structure. The Curie temperature is f
ound to increase monotonically from a critical temperature, T-c equal
to 471 K for the x = 0 sample, to T-c = 681 K for the x= 5 sample. X-r
ay diffraction measurements of magnetic field oriented powders showed
that all compounds exhibit a room temperature uniaxial anisotropy. Mag
netization measurements show that the magnetic anisotropy of Sm2Fe14Al
3 can be increased substantially by the substitution of even a small q
uantity of Co for Fe. Results are discussed in terms of possible appli
cations of these compounds as particulate recording media.