Av. Petukhov et A. Liebsch, THEORY OF 2ND-HARMONIC GENERATION FROM METAL-SURFACES - FREQUENCY-DEPENDENCE AND PENETRATION DEPTH OF SURFACE ANISOTROPY OF AL(111), Surface science, 320(1-2), 1994, pp. 120000051-120000056
A microscopic calculation of the anisotropic nonlinear optical surface
response of Al(111) is reported. The tangential surface current is sh
own to have a remarkably large penetration depth. The anisotropy coeff
icient exhibits a striking variation with frequency and its magnitude
is comparable to the isotropic component in agreement with recent expe
riments.