J. Lovelock, A GEOPHYSIOLOGISTS THOUGHTS ON THE NATURAL SULFUR CYCLE, Philosophical transactions-Royal Society of London. Biological sciences, 352(1350), 1997, pp. 143-147
The climate depends on the atmospheric abundance of sulphur aerosols a
t all levels up to the stratopause. Volcanoes, combustion and biologic
al emissions all contribute and usually result in cooling. The history
of this topic is lively and goes back at least to the eighteenth cent
ury with Benjamin Franklin's comments on the cooling effects of the su
lphuric acid aerosol from the Icelandic volcano, Laki. Mitchell first
drew attention to the potential cooling effects of combustion aerosols
. Charlson and his colleagues proposed that emissions of dimethyl sulp
hide (DMS) from ocean algae might also be important. More recently, Lo
velock & Kump drew attention to the decline of biological sulphur emis
sions with global warming and the possible consequence of a positive f
eedback on climate change. The geophysiological aspects, which arose f
rom the Gaia hypothesis in the early 1970s, form an important part of
the account that follows.