We present the results of an extensive and sensitive search for neutra
l hydrogen at a redshift of approximately 3.3 in an attempt to observe
and study the properties of the precursors of rich clusters of galaxi
es. We have used the Westerbork Synthesis Radio Telescope to observe,
at 327 MHz, a total solid angle of approximately 32 sq. degrees (to ha
lf power) with a total velocity depth ranging from 2000 to 4000 km/s.
If the neutral fraction of the mass at z approximately 3.3 is sufficie
ntly high one predicts structures with angular scales of a few arcminu
tes and velocity dispersions of less than about 1000 km/s with flux de
nsities of up to 10 mJy at 327 MHz. However, no significant positive d
etections were made at spatial resolutions of 1'-8' and velocity resol
utions of 200-2000 km/s at a level of 4-8 mJy. This excludes the exist
ence of neutral H I masses of greater-than-or-similar-to 1-6 x 10(13)h
-2M. (for OMEGA(0) = 1) at comoving number densities exceeding approxi
mately 1000h3Gpc-3. Our upper limits are consistent with and confirm t
he evidence from single lines of sight to quasars from which it follow
s that the fraction of neutral gas must be extremely low out to z appr
oximately 4-5. The implication is that some process (e.g., shock heati
ng and/or the ionizing photon flux from primeval galaxies) has efficie
ntly ionized the majority of the material in forming structures at z a
pproximately 3.3. To be useful, further searches for neutral hydrogen
at high redshift should be conducted at lower frequencies (i.e., highe
r z) and/or considerably higher sensitivity.