T. Wiss et al., RADIATION-DAMAGE IN UO2 BY SWIFT HEAVY-IONS, Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms, 122(3), 1997, pp. 583-588
Specimens of sintered UO2, a high melting point ceramic with the fluor
ite structure, were irradiated with heavy ions (Xe-129, U-238) with di
fferent fluences (5 x 10(10) to 7 x 10(13) ions/cm(2)) acid energies (
173 MeV for Xe ions to 2.713 GeV for U ions). The influence of the ele
ctronic energy loss on the mechanisms of damage formation was studied
in the range of 29 to 60 keV/nm. Transmission Electron Microscopy (TEM
) was performed to identify and characterize the damage induced by the
se ions. Tracks produced by U ions of 2713 and 1300 MeV and by Xe ions
of 173 MeV were observed, The radii of the observed tracks were calcu
lated using a thermal-spike model, taking into account the thermodynam
ic parameters of the material and the energy and velocity of the incom
ing ions. The TRIM code was used to determine the displacement profile
and the energy distribution along the ion paths. Good agreement with
the experimental results was found. The dependence of damage formation
on the ion dose was also studied. For instance, defect clusters and l
oops were produced in UO2 irradiated with Xe-129 of 173 MeV (dE/d x si
milar to 29 keV/nm) between 7 x 10(10) and 7 x 10(13) ions/cm(2).