Aluminum-silicon solid solutions have been prepared by high-pressure q
uenching. Differential scanning calorimetry measurements clearly show
that they are in a non-equilibrium state. Low-temperature specific hea
t and inelastic neutron scattering experiments provide evidence for a
large softening of the transverse acoustic phonon modes, which appears
as the signature of a lattice instability. This shows that it is poss
ible to heavily destabilize the fcc structure of aluminum. This sugges
ts a route to investigate solid-state amorphization of a crystalline s
olid solution.