We present new experimental results on the thermal conductivity of iso
topically enriched C-12 diamond crystals at low temperatures. To our k
nowledge, the measured value for a 99.9% C-12 crystal at 104 K, 410 W/
cm K, is the highest measured thermal conductivity for a solid above l
iquid nitrogen temperature. Our measured temperature dependent conduct
ivities for the isotopically enriched diamond and natural abundance di
amond specimens are well described by Callaway's theoretical model. We
predict that the thermal conductivity of a 99.999% C-12 diamond cryst
al should exceed 2000 W/cm K at approximately 80 K.