Epitaxial LiTaO3 thin films having excellent crystalline properties ha
ve been achieved on (0001)-sapphire substrates using the technique of
pulsed laser deposition. X-ray diffraction analysis revealed that comp
letely single-phase c-oriented LiTaO3 films were produced. X-ray rocki
ng curve analysis showed that the range of misalignment of the c-axis
direction was about 0.2-degrees. Ion channeling studies indicated a mi
nimum backscattering yield of only 4.9%. Channeling also revealed an i
mprovement in crystalline perfection as a function of distance above t
he interface with the sapphire substrate. Optical waveguiding with los
ses on the order of 1 dB/cm was demonstrated.