We report the fourth-harmonic generation of 1.5 ps, 1.053 mu m glass l
aser pulses, where group velocity mismatch plays a significant role, a
t intensities up to 100 GW/cm(2) using newly developed crystal, cesium
lithium berate (CsLiB6O10). Type-I doubler and type-I quadrupler were
used in the fourth harmonic generation experimental scheme. Energy co
nversion efficiencies of 24% and 53% have been achieved for frequency
quadrupling and doubling of the fundamental glass laser pulses, respec
tively. (C) 1996 American Institute of Physics.