We report the detection of atomic carbon in a sample of eight southern
hemisphere high Galactic latitude molecular clouds, using the Antarct
ic Submillimeter Telescope and Remote Observatory. The 492 GHz (P-3(1)
--> P-3(0)) transition of [C I] was detected in all of the clouds obs
erved. The C/CO column density ratio ranges from 0.4 to 2.5 and is sim
ilar to the values previously measured in high-latitude clouds MBM 12
and HT) 210121. For all 10 high-latitude clouds observed in [C I], C/C
O averages similar to 1.2 and decreases with increasing total gas colu
mn density N-H, as predicted by translucent cloud models. Quantitative
comparison with chemical models of homogeneous clouds is unsatisfacto
ry, however, and we conclude that the clumpy structure of clouds must
be taken into account in order to interpret the data properly.