T. Lee et al., 1ST DETECTION OF FALLOUT CS-135 AND POTENTIAL APPLICATIONS OF CS-137 CS-135 RATIOS/, Geochimica et cosmochimica acta, 57(14), 1993, pp. 3493-3497
All three cesium isotopes, natural Cs-133 (stable) plus fission Cs-135
(half-life 2.3 Ma) and Cs-137 (half-life 30 y), were measured in two
coastal sediment samples using our thermal ionization mass spectromete
r equipped with a retarding potential quadrupole lens filter. The Cs-1
35/Cs-133 ratio was about 1 X 10(-9) while Cs-137/Cs-135 was about 0.5
owing to the decay during the past 30 years from their production rat
io of about 1. This appears to be the first detection of fallout Cs-13
5 in nature. Being an isotope ratio, Cs-137/Cs-135 is a far more power
ful chronometer-tracer than Cs-137 alone. In order to explore its pote
ntial, we present briefly two simple models to illustrate how this rat
io may be used to quantitatively estimate recent sedimentation and ero
sion rates.