The ternary alloy Tb0.3Dy0.7Fe2 (Terfenol-D) is of significant technol
ogical interest as it possesses the largest known magnetostriction to
anisotropy ratio near room temperature. Results of microstructural and
magnetic domain observations by Lorentz microscopy and reflection x-r
ay topography are presented from both stoichiometric twinned single cr
ystals prepared by a free-standing zoning technique, and pseudo single
crystals prepared by the Czochralski method. Direct evidence of wall
interactions with dislocations, twin boundaries and precipitates are p
resented which demonstrate the complex interaction between the magneti
c and strain energies within this material.