We measured the third-order nonlinear optical susceptibility chi(3) fo
r C60 and C70 SolUtions as a function of concentration using degenerat
e four-wave mixing with picosecond pulses at 532 nm. From the observed
minimum we were able to obtain the real and imaginary parts of chi(3)
. The real part is negative at this wavelength. Values of the real and
imaginary components of the molecular hyperpolarizability (gamma) cal
culated are in the range 10(-31) esu.