An extensive network of bottle/funnel collectors was used to measure h
ydrologic, SO42- and NO3- fluxes in rain events and in throughfall ben
eath the canopies of several high elevation forest stands in the Great
Smoky Mountains National Park during 1989-1990. The throughfall fluxe
s were used as deposition surrogates to quantify trends in atmospheric
inputs to sapling trees growing in forest gaps and to the mature fore
st canopy at the edge surrounding each gap. The paired gap/edge stands
were located above (1940 m) and below (1720 m) the base of the clouds
typically impacting this mountain. Total hydrologic and ion fluxes be
neath the edge trees during the forest growing season exceeded fluxes
beneath the adjacent gap saplings by nearly a factor of three (eg. 230
vs 88 meq m-2 for SO42-) at both elevations. Water and SO42- fluxes w
ere up to two times greater beneath the forest edge at the cloud-prone
1940 m site than at 1720 m (e.g. 230 vs 110 meq m-2 for SO42-). Howev
er, throughfall NO3- fluxes were about 30% higher at 1720 m (17 vs 13
meq m-2), because this lower site receives greater dry deposition of H
NO3 due to its ridgetop location and greater wind penetration. Estimat
es of SO24- deposition from cloud impaction were consistent with the n
et throughfall flux of SO42- (throughfall flux minus rain flux) at the
1940 m forest edge, but greatly exceeded the net throughfall flux at
1940 m gap, suggesting differences in ion concentrations in cloud drop
lets impacting on mature edge trees and young saplings in forest gaps.