The organic superconductor kappa-(BEDT-TTF)2Cu(SCN)2 shows a region of
negative magnetoresistance (NM) just above the upper critical field.
In order to gain further information about this effect, we have studie
d its dependence on a number of parameters. The magnetoresistance has
been measured as a function of field direction, sample temperature and
current configuration. The temperature dependence of the resistance h
as also been studied as a function of field applied at different angle
s and with different current configurations The NM is found to be much
more pronounced when the measuring current is in the inter-layer dire
ction (j parallel-to a) and almost absent when the current is in the
plane of molecular layers (j perpendicular-to a). This suggests that
the NM is associated with carrier localisation in the inter-layer dire
ction. However, for the former current orientation, the strongest NM i
s observed when the magnetic field is in the inter-layer direction (i.
e. j parallel-to B).