Self-assembled chromophoric multilayers having large second-order opti
cal nonlinearities can be combined with linear guiding materials such
as polymethylmethacrylate to produce two-component frequency doubling
waveguides, This approach introduces considerable flexibility in optim
izing the trade-off between the overlap of waveguide mode profiles and
linear absorption. Extremely low waveguide propagation losses can be
achieved because electric field poling and the accompanying poling-ind
uced optical scattering are obviated. (C) 1997 American Institute of P
hysics.