V. Krylov et al., Femtosecond stimulated Raman scattering in pressurized gases in the ultraviolet and visible spectral ranges, J OPT SOC B, 15(12), 1998, pp. 2910-2916
We investigate femtosecond stimulated Raman scattering (SRS) in H-2, D-2, H
D, and CH4 excited with 300-fs-duration pulses at 390-nm wavelength and wit
h as much as 0.1 mJ of energy. We show that the SRS-generation threshold an
d conversion efficiency are due to the transient nature of SRS in femtoseco
nd regime. We determine optimal conditions for efficient generation in the
broad spectral range 289-797 nm and show how self-phase modulation and whit
e-light generation Limit the ultimate conversion efficiency. (C) 1998 Optic
al Society of America [S0740-3224(98)00912-6] OCIS codes: 190.2620, 190.565
0, 190.5890.