Va. Levchenko et al., MEASUREMENTS OF THE (CO2)-C-14 BOMB PULSE IN FIRN AND ICE AT LAW-DOME, ANTARCTICA, Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms, 123(1-4), 1997, pp. 290-295
(CO2)-C-14 produced in tile atmosphere by nuclear weapons testing in t
he 1960's is now incorporated in the air bubbles of Antarctic ice, The
high atmospheric radiocarbon growth rates through the period of tests
and subsequent decline provide a unique and independent test for the
smoothing of atmospheric CO2 signals due to firn diffusion and bubble
close off, The level of smoothing quantifies the time resolution with
which atmospheric trace gas histories can be reconstructed from ice co
res, In this paper, the methodologies for the preparation and AMS meas
urements of ice core and firn (CO2)-C-14 from high accumulation sites
at Law Dome are detailed, The results are compared with predictions of
a numerical model incorporating firn air diffusion and bubble close-o
ff. The sample sizes, precision of measurements and sources of contami
nation are discussed for both firn and ice samples.