Observations of (CO)-O-18, (HCO+)-C-13, and DCO+ toward 23 low-mass cores a
re used to constrain the fractional ionization (electron abundance) within
them. Chemical models have been run over a wide range of densities, cosmic-
ray ionization rates, and elemental depletions, and we find that we can fit
20 of the 23 cores for densities of n(H2) = (1-3) x 10(4) cm(-3), moderate
C and O abundance variations, and a cosmic-ray ionization rate of zeta(H2)
= 5 x 10(-17) s(-1). The derived ionization fractions lie within the range
10(-7.5) to 10(-6.5), with a median value of x(e,m) = 9 x 10(-8) and typic
al errors for each individual core equal to a factor of 3. These Values imp
ly that the cores are weakly coupled to the magnetic held and that MHD wave
s can propagate within them. The ambipolar diffusion timescale is about an
order of magnitude greater than the free-fall time, and the cores can be co
nsidered to be in quasi-static equilibrium. There is no significant differe
nce between the ionization fraction for cores with and without embedded sta
rs, which suggests that the molecular ionization in cores is primarily gove
rned by cosmic rays alone.