A reflection and transmission technique is described, which allows the dete
rmination of the absorption coefficient spectrum, the refractive index disp
ersion, and the thickness of thin films on transparent substrates. The meth
od may be used at any angle of incidence for s-polarized or p-polarized lig
ht. The absorption spectrum and the refractive index spectrum of a neat rho
damine 6G dye film on a fused silica substrate are determined. The absorpti
on cross-section spectrum of the film is compared with the monomeric dye ab
sorption cross-section spectrum in highly diluted solution. (C) 1998 Elsevi
er Science B.V. All rights reserved.